Laser Spectroscopy of Highly Vibrationally Excited Molecules

This book contains a comprehensive study of both the experimental and theoretical aspects of the basic photophysical interactions that occur in these processes. It first focuses on the nonlinear interaction between the resonant vibrational mode and the intense infrared field and then examines the nonlinear interaction between the vibrational modes themselves due to anharmonicity. The book also discusses related phenomena such as spectra broadening, optical resonance, photon echoes, and dynamical chaos. It includes examples of multiple-photon resonant excitation such as the excitation of OsO4 by COO2 laser radiation, which is detected by the visible luminescence that results.

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